pre-buggy la140 radio-tracer

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    UNCLASSIFIEDAD 406 3061DEFENSE DOCUMENTATION CENTER

    FOR

    SCIENTIFIC AND TECHNICAL INFORMATIONCAMERON STATION, ALEXANDRIA, VIRGINIA

    UNCLASSIFIED

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    NOTICE: When government or other drawings, speci-fications or other data are used for any purposeother than in connection with a definitely relatedgovernment procurement operation, the U. S.Government thereby incurs no responsibility, nor anyobligation whatsoever; and the fact that the Govern-ment may have formmilated, furnished, or in any waysupplied the said drawings, specifications, or otherdata is not to be regarded by implication or other-wise as in any manner licensing the holder or anyother person or corporation, or conveying any rightsor permission to manufacture, use or sell anypatented invention that may in any way be relatedthereto.

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    USNEDL-TR-6384 April 1963

    USE C La140 AS RADIOYRACER IN (PRE-BUGGY) CHMUICAL EXPLOSIONSPreparation and Determination of"lia Its Reaction with Environmental Materials

    - " byO W. B. LaneM. J. Nuckollsw R. M. RaileyC-0JD co

    Ea~CJY-O- m0)\o\ , r 0EH~C3HO\H0.H-I HY~ ~ J

    0) O~c'HH Ed2tOU2~ CdCdt

    043-4-0 C.)d-0

    W o A -i r-i 4

    bD Q) u M C14

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    4o

    9-0SUFCEAE

    80

    440

    3020

    110 10 0010,000PARTICLE DIAMETER (MICRON)

    Fig.- 3 Wet Sieve Anal~rsis

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    TABLE 5Dry Sieve Analysis of Debris From 3rd Row Charge

    Mesh Micron Grams Activity Cumulative CumulativeDiameter Retained (c/m) Mass Activity(% of total) (% of total)

    6 3360 12.97 10,000 85.77 99.414 1190 24.04 55,ooo 61.73 95.848 29 5 34.97 232,000 26.76 81.780 175 12.37 i12,000 14.39 73.9170 88 9.16 123,000 9.16 66.2325 44 3.11 294,000 2.12 47.kPan < 44 2.12 744,000

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    1-4Vi 100 -LiJ> 90--

    r8 0 -

    >60 -050 -

    40

    ,30 -w 0Li

    Li

    S 110- 100 1000 10,000n PARTICLE DIAMETER (MICRON)

    Fig. 4i Dry Sieve Analysis

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    z 90QQ80 -

    70-~60-~50~40-30-w

    UJ

    1i 10101001,0CPARTICLE DIAMETER (MICRON)

    Fig. 5 Sedan Particle Analysis by Wet Sieve

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    TABLE 6Leaching of La 4oFrom Debris by Solutions

    Solution 25 ml 5 Grams Debris %LeachedSolution (c/m)(c/m)

    0.1 N-HC1 79700 199400 40.u621oo 113100 35.5Water 525 206300 0.25415 229700 o.18Seawater 2670 2024o0 1.32166o 224100 0.740.1 N-NaOH 316 187100 0.17

    319 224200 o. 14

    TABLE 7Exchange of Ia 14 From Debris to Clay or to Adobe

    5 g Clay or 5 g Debris % ExchangedAdobe (c/m)(c/m)

    Adobe 102900 47900 68.3lostClay 133000 27800 82.7140500 20000 87.6

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    CONCIJSIONS

    1. Capsules were prepared and delivered as required by the pre-Buggy test schedule.

    2. The capsules contained th e proper amount of la3. Precise sources made possible the calibration of a large-areascintillation counter in units measured by the Victoreen condenser

    r-meter.14o4. The La was distributed on the particles as a function ofsurface area; 90 % of the activity was on sub-sieve (4 44 micron)

    particles which comprised only 8 % of the mass.

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    REFERENCES

    1. I. B. Iane. Some Physical and Radiochemical Measurements of th eDebris from an Underground and Nuclear Detonation. Project SedanReport, PNE 229P (in preparation).

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    Chemistry

    INITIAL DISTRIBUTION

    .CopiesNAVY

    3 Chief, Bureau of Ships (Code 335)1 Chief, Bureau of Ships (Code 320)1 Chief, Bureau of Medicine and Surgery1 Chief, Bureau of Naval Weapons (RRMA-U)2 Chief, Bureau of Yards and Docks (Code 74). Chief, Bureau of Yards and Docks (Code C-400)1 Chief of Naval Operations (Op-07T)1 Chief of Naval Research (Code 104)1 Commander, New York Naval Shipyard (Material Lab.)3 Director, Naval Research Laboratory (Code 2021)2 Director, Naval Research Laboratory (Code 6370)1 Office of Naval Research (Code 422)6 Office of Naval Research, FPO, Ne w York1 CO, U. S. Naval Civil Engineering Laboratory1 OiC, U. S. Naval School (CECOS) Pt. Hueneme1 Chief, Protective Structures Development Center, Fort Belvoir, Va .1 Commander, Naval Air Material Center, Philadelphia1 Naval Medical Research Institute1 U. S. Naval Postgraduate School, Monterey1 Office of Patent Counsel, San Diego1 U. S. Naval Hospital, San Diego

    ARMY

    1 Chief of Research and Development (Atomic Div.)1 Chief of Research and Development (Life Science Div.)1 Deputy Chief of Staff for M ilitary Operations (CBR)1 Chief of Engineers (ENGMC-EB)1 Chief of Engineers (ENGMC-DE)1 Chief of Engineers (ENGCW)6 USA Engineer Nuclear Cratering Group, LRL, Livermore1 CG, Army Materiel Command (AMCRD-DE-NE)1 CG, Ballistic Research Laboratories1 CG, USA CBR Agency1 President, Chemical Corps Board

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    1 CO, Chemical Corps Training Command1 Commandant, Chemical Corps Schools (Library)1 CO , Chemical Research and Development Laboratories1 Commander, Chemical Corps Nuclear Defense Laboratory1 Army Environmental Hygiene Agency1 CG , Aberdeen Proving Ground1 Director, Walter Reed Army Medical Center1 CG , Combat Developments Command (CDCIR-V)1 CG , Quartermaster Res. and Eng. Command1 Hq., Dugway Proving Ground3 The Surgeon General (MEDNE)1 CG, Engineer Res. and Dev. Laboratory1 Director, Office of Special Weapons Development1 CO, Army Research Office1 CO, Watertown Arsenal1 CG, Mobility Command1 CG, Munitions Command1 CO, Frankford Arsenal1 CG , Army Missile Command

    AIR FORCE1 Assistant Chief of Staff, Intelligence (AFCIN-3B)6 CG, Aeronautical Systems Division (ASAPRD-NS)1 Directorate of Civil Engineering (AFOCE-ES)1 Director, USAF Project RAND1 Commandant, School of Aerospace Medicine, Brooks AF B1 Office of the Surgeon (SUP3.1), Strategic Air Command1 Office of the Surgeon General1 CG, Special Weapons Center, Kirtland AF B1 Director, Air University Library, Maxwell AFB1 Commander, Technical Training Wing, 3415th TTG1 Commander, Electronic Systems Division (CRZT)

    OTHER DOD ACTIVITIES3 Chief, Defense Atomic Support Agency (Library)1 Commander, FC/DASA, Sandia Base (FCDV)1 Commander, FC/DASA, Sandia Base (FCTG5, Library)1 Commander, FC/DASA, Sandia Base (FCWT)2 Office of Civil Defense, Washington2 Civil Defense Unit, Army Library20 Armed Services Technical Information Agency1 Director, Armed Forces Radiobiology Research Institute1 Weapons System Evaluation Group, Dr. H. A. Knapp

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    AEC ACTIVITIES' AND OTHERS1 Research Analysis Corporation100 Director, Division of Biology and Medicine1 Aerojet General, Azusa1 Aerojet General, San Ramon1 Allis-Chalmers Manufacturing Co., Milvaukee1 Allis-Chalmers Manufacturing Co., Washington1 Allison Division - GMC2 Argonne ,Cancer Research Hospital10 Argonne National Laboratory1 Atomic Bomb Casualty Commission1 AEC Scientific Representative, France1 AEC Scientific Representative, Japan3 Atomic Energy Commission, Washington4 Atomic Energy of Canada, Limited4 Atomics International2 Babcock and Wilcox Company2 Battelle Memorial Institute1 Beryllium Corporation1 Borden Chemical Company4 Brookhaven National Laboratory1 Bureau of Mines, Albany1 Bureau of Mines, Salt Lake City1 Chance Vought Corporation1 Chicago Patent Group1 Columbia University (Cropper)1 Combustion Engineering, Inc.1 Combustion Engineering, Inc. (NRD)1 Committee on the Effects of Atomic Radiation1 Defence Research Member1 Denver Research Institute1 Division of Ra w Materials, Washington1 Dow Chemical Company, Rocky Flats3 duPont Company, Aiken1 duPont Company, Wilmington1 Edgerton, Germeshausen and Grier, Inc., Goleta1 Edgerton, Germeshausen and Grier, Inc., Las Vegas1 Fundamental Methods Association1 General Atomic Division2 General Dynamics, Fort Worth2 General Electric Company, Cincinnati4 General Electric Company, Richland1 General Electric Company, San Jose1 General Electric Company, St. Petersburg1 General Scientific Corporation

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    1 General Telephone and Electronic Laboratories, Inc.1 Goodyear Atomic Corporation1 Grand Junction Office1 Hughes Aircraft Company, Culver City1 Iowa State University1 Jet Propulsion Laboratory2 Knolls Atomic Power Laboratory2 Los Alamos Scientific Laboratory (Library)1 Mallinckrodt Chemical Works1 Maritime Administration1 Martin-Marietta Corporation1 Massachusetts Institute of Technology1 Monsanto Chemical Company1 Mount Laboratory1 NASA, Lewis Research Center2 NASA, Scientific and Technical Information Facility1 National Bureau of Standards (Library)1 National Bureau of Standards (Taylor)1 National Lead Company of Ohio1 New Brunswick Area Office1 New York Operations Office1 Nuclear Materials and Equipment Corporation1 Nuclear Metals, Inc.1 Office of Assistant General Counsel fo r Patents4 Phillips Petroleum Company1 Power Reactor Development Company4 Pratt and Whitney Aircraft Division1 Princeton University (White)2 Public Health Service, Washington1 Public Health Service, Las Vegas1 Public Health Service, Montgomery1 Purdue University1 Radiation Applications, Inc.1 Sandia Corporation, Albuquerque1 Sandia Corporation, Livermore1 Technical Research Group1 Tracerlab, Inc., Richmond3 Union Carbide Nuclear Company (ORGDP)4 Union Carbide Nuclear Company (ORNL)1 Union Carbide Nuclear Company (Paducah Plant)1 United Nuclear Cor-poration (NDA)1 U. S. Geological Survey, Denver1 U. S. Geological Survey, Menlo Park1 U. S. Geological Survey, Naval Weapons Plant1 U. S. Geological Survey, Washington1 U. S. Geological Survey, WR Division

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    2 University of California Lawrence Radiation Lab., Berkeley2 University of California Lawrence Radiation Lab., Livermore1 University of California, Los Angeles1 University of Hawaii1 University of Puerto Rico1 University of Rochester (Atomic Energy Project)1 University of Utah1 University of Washington (Donaldson)2 Westinghouse Bettis Atomic Power Laboratory1 Westinghouse Electric Corporation (Rahilly)1 Westinghouse Electric Corporation (NASA)1 Yankee Atomic Electric Company25 Technical Information Extension, Oak Ridge

    USNRDL38 USNRDL, Technical Information Division

    DISTRIBUTION DATE: 15 June 193

    2?

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